In-situ measurement of pyrolysis and combustion gases from biomass burning using swept wavelength external cavity quantum cascade lasersAuthor(s): M. C. Phillips; T. L. Myers; T. J. Johnson; D. R. Weise
Source: Optics Express. 28(6): 8680-8700
Publication Series: Scientific Journal (JRNL)
Station: Pacific Southwest Research Station
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Broadband high-speed absorption spectroscopy using swept-wavelength external cavity quantum cascade lasers (ECQCLs) is applied to measure multiple pyrolysis and combustion gases in biomass burning experiments. Two broadly-tunable swept-ECQCL systems were used, with the first tuned over a range of 2089-2262 cm−1 (4.42–4.79 µm) to measure spectra of CO2, H2O, and CO. The second was tuned over a range of 920-1150 cm−1 (8.70–10.9 µm) to measure spectra of ammonia (NH3), ethene (C2H4), and methanol (MeOH). Absorption spectra were measured continuously at a 100 Hz rate throughout the burn process, including inhomogeneous flame regions, and analyzed to determine time-resolved gas concentrations and temperature. The results provide in-situ, dynamic information regarding gas-phase species as they are generated, close to the biomass fuel source.
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CitationPhillips, M. C.; Myers, T. L.; Johnson, T. J.; Weise, D. R. 2020. In-situ measurement of pyrolysis and combustion gases from biomass burning using swept wavelength external cavity quantum cascade lasers. Optics Express. 28(6): 8680-8700. https://doi.org/10.1364/OE.386072.
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